Currently Being ModeratedMay 30, 2012 12:52 PM (in response to Becky Hoop)
How you delete content from your iPod depends on how it is set up to sync with your iTunes library whether that be automatically or manually.
If it's automatically, you must reconfigure your settings so that the album you wish to remove is no longer configured to sync to your iPod. For example, if the Sync only checked songs and videos option is enabled from under the iPod's Summary tab, make sure all the tracks for this album do NOT have a tick mark next to them in your iPod. Then resync your iPod with iTunes.
Otherwise, if you manually manage your iPod's contents, you must manually remove content from it. You can do this by plugging your iPod in and clicking the small black triangle next to your iPod from under the Devices section in the left hand pane of iTunes. This will open up a submenu of content, so go ahead and click on Music. Locate the track or tracks you wish to delete. Highlight them and hit the Delete key or choose Edit -> Delete.