HT202636: Tips for managing your iBooks library and storage on iOS devices
Learn about Tips for managing your iBooks library and storage on iOS devices
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Helpful answers
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May 12, 2013 11:23 PM in response to BVK.balaby King_Penguin,The 'sync collections' setting won't copy content between your devices, all it does is if you move an ibook/epub/PDF into a collection in iBooks on one device, then if that item is also already on the other device then it will moved into the same collection on that other device.
If they are ibooks and they are still in the store then you should be able to re-download them on the second device via the Purchased tab in the ibookstore in the iBooks app. If they are not ibooks (e.g. epubs or PDFs) or they are no longer in the store, then you should be able to copy them from the device to the Books section of your computer's iTunes library via File > Devices > Transfer Purchases and you can then sync them to your other device.