HT5824: Reset iCloud Documents & Data
Learn about Reset iCloud Documents & Data
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Helpful answers
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Mar 5, 2014 1:17 PM in response to shaggie09by randers4,Music available from the iTunes store is already in iCloud (assuming it is still available in the iTunes store). All you would need to do is delete it from your phone and you will see iCloud download symbols to redownload it, as long as you have Music turned on in Settings>iTunes & App Store under Show All.
Music from other sources, such as your CDs, can only be made available in iCloud by subscribing to iTunes Match (http://www.apple.com/itunes/itunes-match/).