HT204545: iTunes: Unable to sync photos
Learn about iTunes: Unable to sync photos
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Helpful answers
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Oct 9, 2013 9:26 PM in response to lysettelozano01by David Shanahan,This usually means you need to restore/reset the phone using iTunes:
http://support.apple.com/kb/HT1414
If that doesn't work then try the HT1808 document linked to in the above document under "Additional Information" heading, i.e. a recovery mode restore.