Pick the song, in the library window, and then hit the delete key. Then you will be asked if you want to move it to trash or keep it in the folder. I always keep mine in the folder in case I want to add it back to library again later.
Select the song and click the delete button. It will ask if you are sure you want to delete it, and you click yes. You could also right click on the song/video and click clear. It will ask you the sme question.
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Taking vidieos out of itune
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