Old iPod Music transfer: G2 to G5
iPod touch (2nd generation), iOS 4.2, the G2 is old but still works
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iPod touch (2nd generation), iOS 4.2, the G2 is old but still works
Your iPods are iPod touch models, correct? That's an important distinction...
iTunes syncing is generally on one direction, from iTunes library to iPod. You cannot use iTunes to transfer song files from iPod to computer (except for songs purchased from the iTunes Store). However, there are third-party utilities that can transfer from iPod to computer. If you do an Internet search on something like "ipod touch transfer," you should get some relevant links. NOTE: Some of the methods that work for "regular" iPods, do not work with iPod touch.
Old iPod Music transfer: G2 to G5