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May 10, 2015 9:55 AM in response to horse202noxby FoxFifth,See the quote below from Sync photos to your iPhone, iPad, and iPod touch in iTunes - Apple Support
If you can't do the following from step 3 then you may be able to do the item below step 4
To delete all synced photos, deselect "Sync Photos from" and, when asked, click "Remove photos."
Delete synced photos
- In iTunes, locate and click on your device.
- Click Photos.
- Choose "Selected albums" and deselect the albums or collections you want to delete.
To delete all synced photos, deselect "Sync Photos from" and, when asked, click "Remove photos." - Click Apply.
Learn how to delete photos and video synced from iTunes when you can't access the originals.