How do I remove videos from Event Library

There are two ways:

Method 1:

Open your Finder

Open the "Movies" folder

Open "iMovie Events" folder

You'll see folders corresponding to your events. Choose which files to delete.

Method 2:

In your iMovie event, Control-click on the video you want to delete

Select Reveal in Finder

You can then delete the video file from there

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You may be aware already, but just to remind you, any clips deleted from an event that are used in a project will affect the project.