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Sep 26, 2015 1:10 PM in response to Appledumdumby FoxFifth,You remove them by syncing again but change the settings/selection on the Photos page of iTunes before doing the sync. Instructions below are from Sync photos from your computer to your iOS device using iTunes - Apple Support
Delete synced photos
- In iTunes, locate and click on your device.
- Click Photos.
- Choose "Selected albums" and deselect the albums or collections you want to delete.
- To delete all synced photos, deselect "Sync Photos from" and, when asked, click "Remove photos."
- Click Apply.