I also tried this:
I had trouble with the symlinker app. It's much better to create symbolic links from the command line. A symbolic Link is like an "alias" or a "shortcut" except that it works at a deeper level in the OS, so it totally fools applications into thinking it's a folder.
There are GarageBand and Logic folders in /Library/Application Support on your boot drive that you will want be redirected to your desired target drive. You do this by creating symbolic links that redirect any read or write by apps to more spacious locations on what we'll call your target drive. Logic will thus go to your target drive to use loops etc, and when it downloads loops etc from Apple it will store them there. A symbolic link can make your target drive look like part of your boot drive.
In my case I have a big spacious drive called BIG where I have a top level folder called /Library, where I've built an Application Support folder into which I've copied the Logic and the GarageBand folders from the boot drive's /Library/Application Support folder. So let's look at how we make this location on BIG replace the one on the overly crowded boot drive.
Start by finding these folders in /Library/Application Support on your boot drive.
After copying them to your target drive, rename the original folders on the boot drive to GarageBand.NOT and Logic.NOT. This is temporary. That way if something goes wrong you can delete any symlinks and name the folder back by removing the .NOT at the end of the name, and it will be like before. Ok so far? Later we'll delete these extras.
Then the symlinks will be built on the boot drive using these two command lines (you will be asked your password). Note that the syntax lists the "target" of the symlink followed by its location, i.e. the "source".
sudo ln -s "/Volumes/BIG/Library/Application Support/Logic” “/Library/Application Support/Logic"
sudo ln -s "/Volumes/BIG/Library/Application Support/GarageBand” “/Library/Application Support/GarageBand"
But it didn't work...
In /Library/Application Support you will now see the 2 symlinks. They look like folders with a little arrow, and if you navigate through them with the finder you will land in the content on the BIG drive.